EPR and magnetism of the nanostructured natural carbonaceous material shungite     

Maria Aldona Augustyniak-Jabłokow  Yurii V. Yablokov  Bartłomiej Andrzejewski  Wojciech Kempiński  Szymon Łoś  Krzysztof Tadyszak  Mikhail Y. Yablokov  Valentin A. Zhikharev 《Physics and Chemistry of Minerals》2010,37(4):237-247

The X-band EPR and magnetic susceptibility in the temperature range 4.2–300 K study of the shungite-I, natural nanostructured material from the deposit of Shunga are reported. Obtained results allow us to assign the EPR signal to conduction electrons, estimate their number, N _P, and evaluate the Pauli paramagnetism contribution to shungite susceptibility. A small occupation (~5%) of the localized nonbonding π states in the zigzag edges of the open-ended graphene-like layers and/or on σ (sp ^2+x ) orbitals in the curved parts of the shungite globules has been also revealed. The observed temperature dependence of the EPR linewidth can be explained by the earlier considered interaction of conduction π electrons with local phonon modes associated with the vibration of peripheral carbon atoms of the open zigzag-type edges and with peripheral carbon atoms cross-linking different nanostructures. The relaxation time T ₂ and diffusion time T _D are found to have comparable values (2.84 × 10⁻⁸ and 1.73 × 10⁻⁸ s at 5.2 K, respectively), and similar dependence on temperature. The magnetic measurements have revealed the suppression of orbital diamagnetism due to small amount of large enough fragments of the graphene layers.  相似文献   

Distribution of compact object mergers around galaxies     

Tomasz Bulik  Krzysztof Belczy&#;ski  Wojciech Zbijewski 《Monthly notices of the Royal Astronomical Society》1999,309(3):629-635

Compact object mergers are one of the currently favoured models for the origin of gamma-ray bursts (GRBs). The discovery of optical afterglows and identification of the nearest, presumably host, galaxies allow the analysis of the distribution of burst sites with respect to these galaxies. Using a model of stellar binary evolution we synthesize a population of compact binary systems which merge within the Hubble time. We include the kicks in the supernovae explosions and calculate orbits of these binaries in galactic gravitational potentials. We present the resulting distribution of merger sites and discuss the results in the framework of the observed GRB afterglows.  相似文献